ArticleACS photonics2026
Standoff Time-Resolved SECARS on Ag-Decorated Silicon Nanowires.
Article in ACS photonics, 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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Abstract
Surface-enhanced coherent anti-Stokes Raman scattering (SECARS) has been widely explored for ultrasensitive vibrational spectroscopy, primarily in microscopy configurations employing high-numerical-aperture optics. Here, we demonstrate standoff detection of molecular vibrational fingerprints using plasmon-enhanced time-resolved SECARS at a working distance of 20 cm. We employ Ag-decorated silicon nanowires as a plasmonic substrate supporting the analyte molecules. Broadband pump (575 nm) and Stokes (625 nm) femtosecond pulses together with a narrowband delayed probe (515 nm) are used to generate the SECARS signal, with excitation and anti-Stokes wavelengths overlapping the plasmonic response of the substrate. System performance is first calibrated through Raman and CARS measurements of liquid pyridine and compressed Na
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