ArticleChemical science2026
Amorphization-enabled decoupling of hydrogen and hydroxide binding on RuSi for efficient alkaline hydrogen evolution.
Article in Chemical science, 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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Abstract
Catalyst optimization for the alkaline hydrogen evolution reaction (HER) is fundamentally constrained by scaling relations between hydrogen binding energy (HBE) and hydroxide binding energy (OHBE), yet rational design strategies capable of synergistically optimizing both descriptors have remained experimentally elusive. Herein, we demonstrate that independent regulation of HBE and OHBE dramatically accelerates alkaline HER kinetics by employing a structurally flexible amorphous RuSi (a-RuSi) as a dual-site model catalyst. Through annealing-induced evolution of structural order and local Ru-Si coordination, the adsorption energetics of H* and OH* are decoupled, which breaks the conventional scaling relationship and shifts the catalytic activity maximum to a higher-performance regime. The disordered structure generates diverse Ru
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