ArticleChemical science2026
Excited-state triplet-doublet spin dynamics in compact donor-acceptor-radical triads.
Article in Chemical science, 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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Abstract
Compact naphthalimide-based donor-acceptor-radical triads, together with their corresponding radical-free donor-acceptor dyads, were prepared as a tunable platform for manipulating long-lived excited-state spin dynamics in closely coupled organic multispin systems. Structural analysis and DFT calculations support a compact, orthogonal geometry, which preserves the distinct functions of the donor, acceptor, and radical fragments while keeping them close enough for efficient excited-state interactions. By combining optical spectroscopy with time-resolved electron paramagnetic resonance (TREPR), we observed a consistent progression across the series. The sequence starts from the localized triplet state of the naphthalimide chromophore and extends to the donor-containing dyads, where triplet locally excited (
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