ArticleScience advances2026
Intramolecular charge redistribution of phosphate anions enabling ultrahigh-voltage lithium metal battery of 600 Wh kg
Shenghang Zhang, Fanteng Meng, Lixuan Yang, Hongquan Liu, Xiaofan Du, Xiangchun Zhuang, Bin Xie, Shitao Wang, Lixin Qiao, Jun Ma and 9 more
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In one paragraphArticle in Science advances, 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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5 · Who and what moneyAuthors and funding
19 authors.
Shenghang ZhangQingdao Industrial Energy Storage Research Institute, Qingdao New Energy Shandong Laboratory, Qingdao Institute of Bioenergy and Bioprocess Technology, Chinese Academy of Sciences, Qingdao 266101, P. R. China.ORCID 0009-0003-8245-9092 Fanteng MengQingdao Industrial Energy Storage Research Institute, Qingdao New Energy Shandong Laboratory, Qingdao Institute of Bioenergy and Bioprocess Technology, Chinese Academy of Sciences, Qingdao 266101, P. R. China.ORCID 0009-0006-9389-0381 Lixuan YangQingdao Industrial Energy Storage Research Institute, Qingdao New Energy Shandong Laboratory, Qingdao Institute of Bioenergy and Bioprocess Technology, Chinese Academy of Sciences, Qingdao 266101, P. R. China.
Hongquan LiuQingdao Industrial Energy Storage Research Institute, Qingdao New Energy Shandong Laboratory, Qingdao Institute of Bioenergy and Bioprocess Technology, Chinese Academy of Sciences, Qingdao 266101, P. R. China.
Xiaofan DuQingdao Industrial Energy Storage Research Institute, Qingdao New Energy Shandong Laboratory, Qingdao Institute of Bioenergy and Bioprocess Technology, Chinese Academy of Sciences, Qingdao 266101, P. R. China.ORCID 0000-0002-7415-6791 Xiangchun ZhuangQingdao Industrial Energy Storage Research Institute, Qingdao New Energy Shandong Laboratory, Qingdao Institute of Bioenergy and Bioprocess Technology, Chinese Academy of Sciences, Qingdao 266101, P. R. China.
Bin XieQingdao Industrial Energy Storage Research Institute, Qingdao New Energy Shandong Laboratory, Qingdao Institute of Bioenergy and Bioprocess Technology, Chinese Academy of Sciences, Qingdao 266101, P. R. China.
Shitao WangQingdao Industrial Energy Storage Research Institute, Qingdao New Energy Shandong Laboratory, Qingdao Institute of Bioenergy and Bioprocess Technology, Chinese Academy of Sciences, Qingdao 266101, P. R. China.
Lixin QiaoQingdao Industrial Energy Storage Research Institute, Qingdao New Energy Shandong Laboratory, Qingdao Institute of Bioenergy and Bioprocess Technology, Chinese Academy of Sciences, Qingdao 266101, P. R. China.ORCID 0000-0003-1892-5477 Jun MaQingdao Industrial Energy Storage Research Institute, Qingdao New Energy Shandong Laboratory, Qingdao Institute of Bioenergy and Bioprocess Technology, Chinese Academy of Sciences, Qingdao 266101, P. R. China.ORCID 0000-0001-5016-8096 Shanmu DongQingdao Industrial Energy Storage Research Institute, Qingdao New Energy Shandong Laboratory, Qingdao Institute of Bioenergy and Bioprocess Technology, Chinese Academy of Sciences, Qingdao 266101, P. R. China.ORCID 0000-0002-2493-3556 Chung-Kai ChangNational Synchrotron Radiation Research Center, Hsinchu 300092, Taiwan, Republic of China.ORCID 0000-0003-0039-1059 Yu-Chun ChuangNational Synchrotron Radiation Research Center, Hsinchu 300092, Taiwan, Republic of China.ORCID 0000-0002-2879-5381 Chang-Yang KuoNational Synchrotron Radiation Research Center, Hsinchu 300092, Taiwan, Republic of China.ORCID 0000-0003-1968-8020 Chien-Te ChenNational Synchrotron Radiation Research Center, Hsinchu 300092, Taiwan, Republic of China.
Zili CuiQingdao Industrial Energy Storage Research Institute, Qingdao New Energy Shandong Laboratory, Qingdao Institute of Bioenergy and Bioprocess Technology, Chinese Academy of Sciences, Qingdao 266101, P. R. China.ORCID 0000-0001-8677-8304 Gaojie XuQingdao Industrial Energy Storage Research Institute, Qingdao New Energy Shandong Laboratory, Qingdao Institute of Bioenergy and Bioprocess Technology, Chinese Academy of Sciences, Qingdao 266101, P. R. China.ORCID 0000-0001-8810-7061 Guanglei CuiQingdao Industrial Energy Storage Research Institute, Qingdao New Energy Shandong Laboratory, Qingdao Institute of Bioenergy and Bioprocess Technology, Chinese Academy of Sciences, Qingdao 266101, P. R. China.ORCID 0000-0001-5987-7569 Funding
No grant is acknowledged in the PubMed record.
6 · The paper itselfAbstract
The advancement of ultrahigh-voltage lithium metal batteries (LMBs) is hindered by the lack of efficient guidelines for electrolyte material development, with current approaches still largely relying on inefficient trial-and-error methods. Herein, we report a high-performance additive design and screening strategy. A library of phosphorus-centered candidates (containing 15,200 molecules) is constructed by simultaneously introducing electron-withdrawing and electron-donating groups to induce intramolecular charge redistribution and tune the electrochemical properties of the molecules. Through unsupervised machine learning-assisted screening, lithium diperfluoropinacolatophosphate (LiDPFP) is identified as the optimal candidate. LiDPFP features localized electron-deficient and electron-rich regions, which tune interfacial reactivity and enhance lithium ion (Li
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PMID42826190
PMCPMC13632741
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