ArticleChemistryOpen2026
Conformational Control of Excited-State Properties in Ortho-Linked Triarylamine-Based Donor-Acceptor Conjugates.
Article in ChemistryOpen, 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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Abstract
A series of intensely blue-emissive ortho-linked donor-acceptor conjugates comprising triarylamine donors and cyanopyridine or benzonitrile acceptors was readily synthesized via the bromine-lithium exchange-borylation-Suzuki (BLEBS) sequence in moderate to good yields. The modular synthetic approach enables systematic variation of conformational constraint as a molecular design element for tailoring excited-state properties. Cyclic voltammetry reveals irreversible dimerization of triarylamine derivatives lacking para-substituents. Photophysical studies in the solid state, solution, and polymethylmethacrylate (PMMA) matrix reveal photoluminescence quantum yields (PLQY) of up to 70%, emission bandwidths as narrow as 2480 cm
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