ArticleNature communications2026
Programmable mesoporous carbon architectures from liquefied wood via reactive-emulsion-mediated self-assembly.
Article in Nature communications, 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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13 authors.
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Abstract
Developing biomass-derived programmable self-assembly systems for precise control of carbon morphology and architecture remains challenging, primarily because of the intrinsic heterogeneity that hinders controllable assembly. Here, we report a biomass-enabled reactive-emulsion-mediated strategy for converting liquefied wood into various mesoporous carbon nanomaterials. This synthesis features the introduction of trioctyl phosphate (TOP) as a hydrophobic swelling agent for composite micelles and an interfacial modifier, shifting the preferred micelle curvature/packing tendency and biasing the assembly pathway from homogeneous aqueous self-assembly toward interface-associated anisotropic organization. This coupled regulation progressively reduces the density of ordered mesochannels within the fibrous framework and promotes the evolution from ordered mesoporous nanofibers to hollow nanofibers and bowl-like architectures. The fabricated hollow carbon nanofiber-based mixed ion-electron thermoelectric generator (MTEG) exhibits a high thermopower of 12.33 mV K
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