ArticleACS physical chemistry Au2026
Accelerated OH Oxidation of Methyl Chloride via Surface Accumulation at the Air-Water Interface.
Article in ACS physical chemistry Au, 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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Abstract
Chemical reactions often proceed differently at the air-water interface than in bulk solution. In particular, "on-water" catalysis refers to cases where reactions appear to be accelerated at aqueous surfaces. A growing body of work shows that rate acceleration can arise from intertwined effects, including modified solvation and acid-base behavior, as well as enhanced reactant concentrations. Despite this progress, it remains difficult to quantify, for specific atmospheric reactions, how much interfacial rate enhancement arises from (i) intrinsic changes in the free energy barrier versus (ii) concentration-driven effects, because fully converged interfacial free energy profiles are costly to obtain with ab initio molecular simulations. Here, we address this challenge for the reaction of methyl chloride CH
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