ArticleGlobal challenges (Hoboken, NJ)2026
Hybrid NiMn-LDHs as Active Materials for Electro-Oxidation of Organic Pollutants.
Article in Global challenges (Hoboken, NJ), 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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Abstract
Electrochemical oxidation of phenol is a promising route for sustainable treatment of wastewater containing toxic aromatic pollutants, but its practical application is limited by sluggish kinetics and competing anodic side reactions. Here, we report NiMn-based layered double hydroxide electrocatalysts (NiMn-LDH) that enhance phenol degradation under mild electrochemical conditions. Mn incorporation into the LDH structure provides accessible higher oxidation states, improving redox flexibility, promoting hydroxyl radical (·OH) generation, and suppressing the competing oxygen evolution reaction. Three variants, NiMn-LDH-CNT, NiMn-LDH-CMC, and NiMn-LDH-Tris, were synthesized to assess the influence of conductive additives and synthesis media. The CNT-supported catalyst showed the highest activity, achieving >95% phenol removal within minutes at current densities up to 20 mA cm
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