ArticleScience advances2026
Amine-rich cross-linking templates enabling toughened self-assembled monolayer for stable perovskite solar modules.
Zhinan Zhang, Sifan Chen, Chuan Peng, Yinghao Xu, Shaofu Wang, Wenbo Li, Yang Zheng, Wei Wang, Shengjie Du, Fuyi Zhou and 6 more
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16 authors.
Zhinan ZhangSchool of Physics and Technology, Key Laboratory of Artificial Micro/Nano Structures of Ministry of Education, Wuhan University, Wuhan 430072 P.R. China.ORCID 0000-0001-8276-1927 Sifan ChenSchool of Physics and Technology, Key Laboratory of Artificial Micro/Nano Structures of Ministry of Education, Wuhan University, Wuhan 430072 P.R. China.
Chuan PengSchool of Physics and Technology, Key Laboratory of Artificial Micro/Nano Structures of Ministry of Education, Wuhan University, Wuhan 430072 P.R. China.
Yinghao XuSchool of Physics and Technology, Key Laboratory of Artificial Micro/Nano Structures of Ministry of Education, Wuhan University, Wuhan 430072 P.R. China.ORCID 0000-0001-6065-5250 Shaofu WangSchool of Physics and Technology, Key Laboratory of Artificial Micro/Nano Structures of Ministry of Education, Wuhan University, Wuhan 430072 P.R. China.
Wenbo LiSchool of Physics and Technology, Key Laboratory of Artificial Micro/Nano Structures of Ministry of Education, Wuhan University, Wuhan 430072 P.R. China.
Yang ZhengSchool of Physics and Technology, Key Laboratory of Artificial Micro/Nano Structures of Ministry of Education, Wuhan University, Wuhan 430072 P.R. China.
Wei WangSchool of Physics and Technology, Key Laboratory of Artificial Micro/Nano Structures of Ministry of Education, Wuhan University, Wuhan 430072 P.R. China.
Shengjie DuSchool of Physics and Technology, Key Laboratory of Artificial Micro/Nano Structures of Ministry of Education, Wuhan University, Wuhan 430072 P.R. China.ORCID 0009-0000-1715-4274 Fuyi ZhouState Key Laboratory of Silicon and Advanced Semiconductor Materials School of Materials Science and Engineering, Zhejiang University, Hangzhou 310027, P.R. China.ORCID 0000-0001-8275-2932 Haimeng XinState Key Laboratory of Silicon and Advanced Semiconductor Materials School of Materials Science and Engineering, Zhejiang University, Hangzhou 310027, P.R. China.ORCID 0009-0000-3792-6833 Sixiong LiSchool of Physics and Technology, Key Laboratory of Artificial Micro/Nano Structures of Ministry of Education, Wuhan University, Wuhan 430072 P.R. China.ORCID 0009-0004-3365-6337 Xingzhong ZhaoSchool of Physics and Technology, Key Laboratory of Artificial Micro/Nano Structures of Ministry of Education, Wuhan University, Wuhan 430072 P.R. China.
Ti WangSchool of Physics and Technology, Key Laboratory of Artificial Micro/Nano Structures of Ministry of Education, Wuhan University, Wuhan 430072 P.R. China.ORCID 0000-0002-6828-7277 Zhenyi NiState Key Laboratory of Silicon and Advanced Semiconductor Materials School of Materials Science and Engineering, Zhejiang University, Hangzhou 310027, P.R. China.ORCID 0000-0002-8379-9182 Zhenhua YuSchool of Physics and Technology, Key Laboratory of Artificial Micro/Nano Structures of Ministry of Education, Wuhan University, Wuhan 430072 P.R. China.ORCID 0000-0002-0832-2384 Funding
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6 · The paper itselfAbstract
As the most popular hole-selective materials in efficient p-i-n perovskite solar cells (PSCs), self-assembled monolayers (SAMs) still remain great challenges in long-term stability due to their frail construction and week bonding. To form a toughened donor-acceptor interface, here, we adopt an amine-rich cross-linking templates for SAM layer growth. The enhanced Coulombic interaction between polymer amines and SAMs promotes the formation of SAM growth networks, resulting in reduced self-aggregation of SAMs and the uniform SAM films with high coverage. This design minimizes substrate exposure and suppresses perovskite degradation. Consequently, the unencapsulated mini-module retains 94.19% of their initial efficiency after aging for 10,190 hours under the ISOS-D-1 condition and 93.37% of their initial efficiency for 744 hours under the ISOS-L-2 condition. The optimized interface and perovskite films minimizes carrier transport loss, which result in the champion efficiency of 27.07 (certified 26.39%), 24.03, and 18.48% for PSC, mini-module and submodule (aperture area of 14.4 and 700 cm
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PMID42758819
PMCPMC13588155
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