ArticleChemical science2026
A silk fibroin hybrid hydrogel electrolyte enables highly robust aqueous zinc-ion batteries to operate from -60 to 60 °C.
Article in Chemical science, 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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Abstract
Aqueous zinc-ion batteries (AZIBs) enable safe and sustainable grid-scale energy storage but are limited by dendrite growth, parasitic reactions, and poor temperature tolerance. Herein, we report a multifunctional silk fibroin/polyacrylamide hydrogel electrolyte (SF/PAM-HGE) enabling stable zinc electrochemistry from -60 to 60 °C. SF β-sheet-mediated network reconstruction enhances the mechanical properties of the hydrogel electrolyte, whereas SF's abundant polar groups disrupt water hydrogen bonds, granting the hydrogel wide-temperature adaptability. In addition, the ligand environment tailored by SF's zincophilic polar groups regulates the Zn
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