ReviewPolymers2026
Perhydropolysilazane as a Precursor for Solution-Processed Silicon-Based Materials: Synthesis, Conversion Routes and Mechanisms, Properties, and Applications.
Review in Polymers, 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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3 authors.
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Abstract
Perhydropolysilazane (PHPS) has attracted considerable attention as a versatile precursor for solution-processed silicon-based materials because of its carbon-free backbone, high chemical reactivity, and compatibility with low-temperature processing. This review provides a comprehensive overview of the synthesis of PHPS, its conversion routes and mechanisms, the structure-property relationships of PHPS-derived materials, and their current and emerging applications. The literature demonstrates that PHPS conversion is governed by coupled hydrolysis, oxidation, nitridation, dehydrogenation, photochemical activation, and reactive-species-mediated processes, resulting in compositionally and structurally diverse silicon-based networks, including SiO
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