ArticleChemical science2026
A DPP2-HHTP-COF interfacial layer enabling ultra-long cycling stability of Sn anodes
Article in Chemical science, 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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3 authors.
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Abstract
Aqueous Sn-air batteries offer the advantages of low cost, high safety, and high theoretical capacity. However, Sn anodes are susceptible to the hydrogen evolution reaction (HER) and "dead Sn" detachment, leading to reversible capacity decay and severely limiting battery performance. Herein, we propose a DPP2-HHTP-COF mediated electron-ion decoupling strategy. An artificial electronically conductive DPP2-HHTP-COF interfacial layer is constructed on the Sn anode. The DPP2-HHTP-COF conjugated framework and electron-accepting units synergistically reconstruct the interfacial electronic structure, forming an electron-deficient layer and increasing the HER energy barrier. Meanwhile, the active coordination sites of the DPP2-HHTP-COF interfacial layer enable selective binding of SnO
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