ArticleAngewandte Chemie (International ed. in English)2026
The Part and the Whole: Field-Dependent THz-EPR Spectroscopy Probes Lattice-Dependent Electronic Structure in Iron(II) Spin Crossover.
Article in Angewandte Chemie (International ed. in English), 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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Abstract
Frequency-domain Fourier-transform (FD-FT) THz-EPR spectroscopy provides direct access to kinetically trapped high-spin (HS) states in iron(II) spin crossover (SCO) complexes. Using temperature-induced excited spin-state trapping (TIESST), the low-temperature electronic structure of the HS state is accessed despite a diamagnetic low-spin (LS) ground state. Field-dependent spectra resolve the splitting of the HS ground-state manifold and provide evidence for spin-phonon coupling, described by an avoided-crossings Hamiltonian supported by ab initio calculations. THz-EPR further quantifies the remaining HS fraction (
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