ArticleACS omega2026
Driving Forces of UCST and LCST Liquid-Liquid Phase Separations.
Article in ACS omega, 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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Abstract
A liquid mixture of two or more components can phase separate into two liquid phases by changing the temperature. Ordinary chemical perception would attribute this transition to a competition between the favorable enthalpy of the biphasic state and the favorable entropy of the (mixed) monophasic state, rationalizing the stability of these states, respectively, at low and high temperatures. This is indeed the case for a UCST liquid-liquid phase separation. However, in contrast, in LCST behavior, the monophasic mixed state is observed at low temperatures, whereas the biphasic state is observed at high temperatures. This perplexing behavior has triggered different hypotheses about mechanisms capable of explaining it. In this paper, we study, by molecular dynamics simulations, two ionic liquids (ILs), [Hbet]-[Tf
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