ArticleNano-micro letters2026
Hotspot to Homogeneous: Amorphous Interfacial Current Redistribution Enables Stable Solid-State Lithium-Metal Batteries.
Article in Nano-micro letters, 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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11 authors.
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Abstract
Interfacial instability in oxide ceramic electrolyte (OCE)-based solid-state lithium metal batteries (SSLMBs) is conventionally attributed to chemical incompatibility or mechanical failure, yet the underlying atomic-scale mechanisms remain elusive. Here, we reveal that grain boundaries (GBs) in polycrystalline OCEs function as bipolar interfacial hotspots, accelerating three degradation pathways: lowering barriers for Li dendrite nucleation and enabling electron-leakage-driven reduction at anode side, while generating localized overpotentials for cathode phase transformation. To deactivate these GB-driven hotspots, we develop a laser-induced amorphization strategy that constructs a GB-free amorphous interlayer capable of homogenizing Li
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