ArticleAngewandte Chemie (International ed. in English)2026
Suppression of Peierls Instability in a Metal-Halide Porous Framework.
Article in Angewandte Chemie (International ed. in English), 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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Abstract
Peierls distortion is a lattice instability in low-dimensional materials driven by electron-phonon coupling, which opens an energy gap at the Fermi level and induces a metal-insulator transition. Suppressing this distortion is crucial for stabilizing metallic and superconducting states in low-dimensional systems, yet achieving such suppression remains challenging without external chemical doping or high-pressure conditions. Metal-organic framework (MOF) forms a periodic porous structure with well-defined channels and functional sites. In this work, we harness the intrinsic periodic electrostatic potential of a porous framework to suppress the Peierls instability in one-dimensional platinum-halide (Pt-X) chains. By integrating Pt-X chains into the ordered nanochannels of the porous material, we achieved suppression of detectable Peierls distortion, as evidenced by the absence of lattice distortion and an approximately four-order-of-magnitude enhancement in its electrical conductivity (from 4.8 × 10
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