ArticleACS omega2026
Microrheological Evolution of C-S-H and M-S-H Gels During Gelation and the Regulatory Mechanism of Cations.
Article in ACS omega, 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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10 authors.
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Abstract
Inorganic silicate gels, including calcium silicate hydrate (C-S-H) gel and magnesium silicate hydrate (M-S-H) gel, exhibit notable advantages in profile control and water shutoff applications in high-salinity oilfields both domestically and internationally. To elucidate the influence of ions on the gelation state and process of silicate gels in high-salinity reservoirs, this study employs diffusing wave spectroscopy (DWS) to investigate the effects of common reservoir cations on the microrheological behavior of C-S-H gel and M-S-H gel. The results indicate that the gelation process of C-S-H gel can be divided into four stages: an initial viscosity-dominated stage; a rapid cross-linking stage (1-2 h) with sharply decreased mean square displacement (MSD) and emerging elastic dominance; a stable equilibrium stage (2-12 h) with stabilized network structure; and a long-term relaxation stage (12-72 h) featuring increased MSD, declining modulus, and local network relaxation. In contrast to C-S-H gel, M-S-H gel consistently exhibits viscosity-dominated fluid behavior throughout the gelation process, with the slope of the MSD curve remaining close to unity, indicating that it does not form a dense elastic network. Cation type exerts a significant regulatory effect on the microrheological behavior of the two silicate gels. For C-S-H gel, Ca
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