ArticleThe journal of physical chemistry. C, Nanomaterials and interfaces2026
Searching for a Correlation between Interfacial Liquid Structure and Hydrodynamic Slip: A Case Study of Water/Silica Interface.
Article in The journal of physical chemistry. C, Nanomaterials and interfaces, 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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Abstract
Hydrodynamic slip at the solid-liquid interface is governed by molecular-scale interactions; however, establishing a direct correlation between interfacial liquid structure and slip behavior is challenging due to the difficulty of isolating nanoscale interfacial structures of water at the solid surface from the bulk water structure. Here, we investigate the relationship between hydrodynamic slip and interfacial water structure at the silica-water interface as a function of NaCl concentration. Vibrational sum-frequency generation (SFG) spectroscopy was used to probe interfacial water structure by deconvoluting Stern-layer and diffuse-layer contributions in the SFG response using the maximum entropy method, and liquid-cell atomic force microscopy was used to quantify the hydrodynamic slip length. Supported by molecular dynamics simulations that resolve molecular orientation and density profiles of water near the silica surface, we identify the distinct hydrogen-bonding configuration and orientation of interfacial water molecules. In the low ionic strength regime (≤10
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