ArticleAngewandte Chemie (International ed. in English)2026
Heterobimetallic Janus Catalysts for the One-Pot Synthesis of Polar-Apolar Block Copolymers.
Article in Angewandte Chemie (International ed. in English), 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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Abstract
The one-pot synthesis of apolar-polar block copolymers combining polyolefins with polyesters has been a long-standing challenge in polymer chemistry. Despite broad-reaching applications of apolar-polar block copolymers in drug delivery, compatibilisation of polymer blends and biomedical materials, their synthesis often requires multi-step protocols with multiple catalysts and several isolation and purification steps. This is a particular challenge when combining the polymerisation of non-activated α-olefins with lactones, as these two distinct polymerisation mechanisms are often incompatible. This work reports heterobimetallic Janus catalysts for orthogonal 1-hexene and ε-caprolactone polymerisation. Generated in situ, the active catalysts combine distinct Ti and Al metal centres connected by a Ti-C(H)═C(R)CH
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