ArticleSmall (Weinheim an der Bergstrasse, Germany)2026
Hierarchical Interfacial Engineering of Boehmite-Coated Separators via Silane Functionalization and Electron-Beam Irradiation.
Article in Small (Weinheim an der Bergstrasse, Germany), 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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Abstract
Interfacial instability at the ceramic-polymer interface in ceramic-coated separators remains a critical challenge, as weak adhesion can cause coating delamination and compromise lithium-ion battery safety and electrochemical performance. Here, we report a dual strategy combining (3-aminopropyl)triethoxysilane (APTES)-functionalized boehmite (AlOOH) with electron-beam (EB) irradiation to reinforce ceramic-coated high-density polyethylene (HDPE) separators. APTES promotes coupling between AlOOH and the poly(acrylic acid) binder, while EB irradiation strengthens the interfacial network. APTES functionalization increases tensile strength from 136.13 to 167.78 MPa and elongation at break from 37.52% to 72.84%. Irradiation at 50 kGy further raises tensile strength to 171.72 MPa while retaining 66.28% elongation. The combined treatments increase peel strength from 118.27 to 257.68 N m
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