ArticleScience advances2026
A complementary descriptor for elucidating selective PMS activation by iron single-atom catalysts with tunable interatomic distances.
Yifei Wang, Xuedi Sun, Hao Wang, Yiyang Wu, Yuqing Ma, Ze Wang, Tingting Zhu, Jinshan Wei, Yang Huo, Meng Sun and 1 more
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In one paragraphArticle in Science advances, 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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11 authors.
Yifei WangNational Engineering Laboratory for Advanced Municipal Wastewater Treatment and Reuse Technology, Key Laboratory of Beijing for Water Quality Science and Water Environment Recovery Engineering, Beijing University of Technology, Beijing 100124, China.ORCID 0000-0002-3386-7677 Xuedi SunNational Engineering Laboratory for Advanced Municipal Wastewater Treatment and Reuse Technology, Key Laboratory of Beijing for Water Quality Science and Water Environment Recovery Engineering, Beijing University of Technology, Beijing 100124, China.
Hao WangNational Engineering Laboratory for Advanced Municipal Wastewater Treatment and Reuse Technology, Key Laboratory of Beijing for Water Quality Science and Water Environment Recovery Engineering, Beijing University of Technology, Beijing 100124, China.
Yiyang WuNational Engineering Laboratory for Advanced Municipal Wastewater Treatment and Reuse Technology, Key Laboratory of Beijing for Water Quality Science and Water Environment Recovery Engineering, Beijing University of Technology, Beijing 100124, China.
Yuqing MaNational Engineering Laboratory for Advanced Municipal Wastewater Treatment and Reuse Technology, Key Laboratory of Beijing for Water Quality Science and Water Environment Recovery Engineering, Beijing University of Technology, Beijing 100124, China.
Ze WangNational Engineering Laboratory for Advanced Municipal Wastewater Treatment and Reuse Technology, Key Laboratory of Beijing for Water Quality Science and Water Environment Recovery Engineering, Beijing University of Technology, Beijing 100124, China.
Tingting ZhuKey Laboratory of Environmental Aquatic Chemistry, State Key Laboratory of Regional Environment and Sustainability, Research Centre for Eco-Environmental Sciences, Chinese Academy of Sciences, Beijing 100085, China.ORCID 0009-0005-2416-4899 Jinshan WeiKey Laboratory of Environmental Aquatic Chemistry, State Key Laboratory of Regional Environment and Sustainability, Research Centre for Eco-Environmental Sciences, Chinese Academy of Sciences, Beijing 100085, China.ORCID 0000-0002-1696-5507 Yang HuoScience and Technology Innovation Center for Municipal Wastewater Treatment and Water Quality Protection, Northeast Normal University, Changchun 130117, China.ORCID 0000-0002-4477-4636 Meng SunKey Laboratory of Environmental Aquatic Chemistry, State Key Laboratory of Regional Environment and Sustainability, Research Centre for Eco-Environmental Sciences, Chinese Academy of Sciences, Beijing 100085, China.ORCID 0000-0002-8188-9264 Jae-Hong KimDepartment of Chemical and Environmental Engineering, Yale University, New Haven, CT 06520-8286, USA.ORCID 0000-0003-2224-3516 Funding
No grant is acknowledged in the PubMed record.
6 · The paper itselfAbstract
The activation of peroxymonosulfate (PMS) for selective oxidant generation in advanced oxidation process is a sought objective when using single-atom catalysts (SACs) over conventional nanomaterials. However, challenges in controlling atomic-level morphology and understanding the intricate interplay between electronic and geometric properties that affect catalytic selectivity hinder rational material design. To address this issue, we developed a library of iron single-atom catalysts (FeSACs) featuring tunable interatomic distances ranging from 2.6 to 10.5 angstroms, facilitating the independent investigation of electronic and geometric effects. We propose a complementary descriptor (CD) integrating electronic effect index (
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PMID42600020
PMCPMC13475614
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