ArticleChemSusChem2026
Facet-Engineered Zn Nanosheet Arrays for High-Energy-Density Fiber-Shaped Zn-Air Batteries.
Article in ChemSusChem, 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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Abstract
Fiber-shaped zinc-air batteries (FZABs) hold great promise for wearable energy storage owing to their intrinsic safety, mechanical flexibility, and high theoretical energy density, yet their practical energy density remains fundamentally constrained by the low utilization of Zn anodes, originating from restricted interfacial accessibility and sluggish reaction kinetics, which lead to incomplete Zn stripping and "dead Zn" accumulation. Here, we address this critical challenge by developing a facet-engineered hierarchical fiber-shaped Zn anode (HF-Zn), in which vertically aligned nanosheet arrays are integrated onto a zincophilic polydopamine (PDA)-modified carbon fiber scaffold. The PDA interfacial layer enables uniform Zn nucleation and homogenized current distribution, directing the growth of (101)-dominant Zn nanosheets with intrinsically fast and reversible stripping/plating kinetics. Coupled with a porous conductive framework that promotes electrolyte penetration and charge transport, this design fundamentally improves Zn utilization. As a result, the assembled FZAB achieves a high specific capacity of 620 mAh g
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