ArticleChemical science2026
From C-C bond cleavage to fluorescence: cyclic (alkyl)(amino)carbene-driven activation of 1,2-diketones.
Article in Chemical science, 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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9 authors.
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Abstract
We report that cyclic (alkyl)(amino)carbenes (CAACs) mediate the selective C-C bond cleavage of 1,2-diketones, thereby establishing reaction-driven structural reorganization as a strategy for creating luminescent aluminum complexes. Leveraging the ambiphilicity of CAACs, nucleophilic attack followed by intramolecular electronic redistribution triggers selective C-C bond cleavage. Subsequent stoichiometric control of AlCl
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