ArticleAdvanced science (Weinheim, Baden-Wurttemberg, Germany)2026
Molecular-Level Pore Engineering for Precise Separation via Active Solvent-Mediated Interfacial Polymerization.
Article in Advanced science (Weinheim, Baden-Wurttemberg, Germany), 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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Abstract
Polymer membranes typically face various selectivity demands in practical separations. Tuning the selectivity largely relies on regulating the pore size and distribution in membranes without disrupting the integrity of the polymer network. While monomer design or additive incorporation shows advances in pore tuning, homogeneous sub-nanometer pore tuning in polymer matrix remains challenging as traditional solvents act solely as diffusive media, leading to uncontrolled polymerization. Here, we report an active solvent-mediated interfacial polymerization strategy that enables molecular-level pore engineering of membrane selective layer. By utilizing the microemulsion, a special solvent, we show that ∼1 nm microemulsions induces localized quasi-homogeneous polymerization, templating molecular-level pores within the polyamide network. The resulting membranes exhibit excellent water permeance of 58.7 L m
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