ArticleJACS Au2026
Metalloradical Activation of Iodonium Ylides for Catalytic Radical Cyclization via Fe(III)-Based Metalloradical Catalysis.
Article in JACS Au, 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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Abstract
Transition metal-catalyzed olefin cyclization via metalloradical catalysis (MRC) is a highly versatile strategy for synthesizing functionalized cyclopropanes and furans. However, mostly diazo compounds have been used as metalloradicophiles for the formation of α-metalloalkyl radical complexes. These compounds suffer from limitations in their use; their explosive or hazardous nature makes them challenging to work with. The most employed catalysts in MRC, Co-(II) porphyrin complexes, are stable in their solid forms in open air, but remain susceptible to oxidation in solution and require inert reaction conditions during catalysis. In this work, we have explored cyclic iodonium ylides as surrogate metalloradicophiles using air-stable Fe-(III)-porphyrin complex, Fe
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