ArticleJACS Au2026
Generalization of Titanocene-Catalyzed Arylation of Epoxides through Radical Polar Crossover by Consecutive Paired Electrolysis.
Article in JACS Au, 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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Abstract
Here, we describe the merging of titanocene-catalyzed radical arylation with electro-organic synthesis that combines the advantages of both fields. The critical mechanistic issue of the titanocene-catalyzed radical arylation, the efficiency of rearomatization by a proton-coupled electron transfer, can be efficiently resolved via a radical polar crossover. This is achieved in a unique manner by consecutive paired galvanostatic electrolysis through a decoupling of the electron and proton transfer steps by spatially separating the critical redox processes, the anodic oxidation of the radical σ-complex to the cationic σ-complex, and the mild
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