Evidence map›Paper›PMID 42527397›Full record

ArticleNature communications2026

Nonmonotonic Screening and Solvation Dynamics of the Electrical Double Layer in Concentrated Lithium Salt Electrolytes.

Xiaoting Yin, Feng Wang, Zengming Zhang, Ru-Yu Zhou, Zhaobin Chen, Tairui Wu, Li Zhang, Jun Huang, Deyin Wu, Jun Cheng and 2 more

Abstract read
In one paragraph

Article in Nature communications, 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.

0numbers the graph read from it
0cells of the map it votes in
0citing papers in PubMed
–field-weighted citation impact
1 · What the graph read from it

What it found

Each row is one number read from the abstract, on the scale the paper reported it, with its interval. Left of the dashed line favours the treatment, right favours the comparator. Under each row is the sentence it came from. New to these charts? A ten-minute tutorial.

The abstract states no effect estimate the extractor could read, or names no intervention and outcome on the map, so this paper lights no cell and moves no belief. It is still indexed, cited and linked below.

2 · The registry

The trial behind it

Trials whose registry record cites this paper, or whose number appears in the abstract. A trial that started after this paper was published is citing it as background, not reporting it.

Neither the registry nor the abstract names a trial number. If this is a trial report, that itself is worth knowing.

3 · Its place in the literature

Who cites it

0 citing papers in PubMed.

No citing paper in PubMed yet.

4 · The record

Corrections and comments

PubMed lists nothing against this paper. Absence here is not a guarantee, only a check that was made.

5 · Who and what money

Authors and funding

12 authors.

Xiaoting Yin *State Key Laboratory of Physical Chemistry of Solid Surfaces, College of Chemistry and Chemical Engineering, Xiamen University, Xiamen, 361005, China.ORCID http://orcid.org/0009-0003-3024-0320
Feng Wang *Laboratory of AI for Electrochemistry (AI4EC), IKKEM, Xiamen, 361005, China.
Zengming ZhangInstitute of Energy and Climate Research, IET-3: Theory and Computation of Energy Materials, Forschungszentrum Jülich GmbH, 52425, Jülich, Germany.
Ru-Yu ZhouState Key Laboratory of Physical Chemistry of Solid Surfaces, College of Chemistry and Chemical Engineering, Xiamen University, Xiamen, 361005, China.
Zhaobin ChenState Key Laboratory of Physical Chemistry of Solid Surfaces, College of Chemistry and Chemical Engineering, Xiamen University, Xiamen, 361005, China.
Tairui WuState Key Laboratory of Physical Chemistry of Solid Surfaces, College of Chemistry and Chemical Engineering, Xiamen University, Xiamen, 361005, China.
Li ZhangState Key Laboratory of Physical Chemistry of Solid Surfaces, College of Chemistry and Chemical Engineering, Xiamen University, Xiamen, 361005, China.ORCID http://orcid.org/0000-0003-0016-2918
Jun HuangInstitute of Energy and Climate Research, IET-3: Theory and Computation of Energy Materials, Forschungszentrum Jülich GmbH, 52425, Jülich, Germany. ju.huang@fz-juelich.de.ORCID http://orcid.org/0000-0002-1668-5361
Deyin WuState Key Laboratory of Physical Chemistry of Solid Surfaces, College of Chemistry and Chemical Engineering, Xiamen University, Xiamen, 361005, China. dywu@xmu.edu.cn.ORCID http://orcid.org/0000-0001-5260-2861
Jun ChengState Key Laboratory of Physical Chemistry of Solid Surfaces, College of Chemistry and Chemical Engineering, Xiamen University, Xiamen, 361005, China. chengjun@xmu.edu.cn.ORCID http://orcid.org/0000-0001-6971-0797
Bingwei MaoState Key Laboratory of Physical Chemistry of Solid Surfaces, College of Chemistry and Chemical Engineering, Xiamen University, Xiamen, 361005, China.
Jiawei YanState Key Laboratory of Physical Chemistry of Solid Surfaces, College of Chemistry and Chemical Engineering, Xiamen University, Xiamen, 361005, China. jwyan@xmu.edu.cn.ORCID http://orcid.org/0000-0002-0045-6169

Funding

Ministry of Science and Technology of the People's Republic of China (Chinese Ministry of Science and Technology) 2023YFA1509001National Natural Science Foundation of China (National Science Foundation of China) 22372140National Natural Science Foundation of China (National Science Foundation of China) 224B2209
6 · The paper itself

Abstract

Understanding the electrical double layer in lithium-ion battery electrolytes is fundamental to improving interfacial processes that govern battery performance and lifetime. However, the microstructure and dynamics of the electrical double layer in highly concentrated lithium salt solutions remain elusive. Herein, combining electrochemical analyses, in situ gap-enhanced Raman spectroscopy and molecular dynamics simulations, we reveal nonmonotonic variation of electrostatic screening with concentration and different exchange kinetics of anions and solvent molecules in the solvation sheath of lithium ions. We find that increasing solvation entropy favors the formation of an anion-rich solvation environment in highly concentrated electrolytes, accelerating Li

Identifiers

PMID42527397
PMCPMC13421668

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