ArticleACS omega2026
Solvent-Free Surface Engineering of Gas Diffusion Electrodes via Initiated Chemical Vapor Deposition for Durable Zinc-Air Batteries.
Article in ACS omega, 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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3 authors.
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Abstract
Gas diffusion electrodes (GDEs) in rechargeable zinc-air (Zn-air) batteries often suffer from catalyst dissolution, electrolyte flooding, and degradation of the gas-liquid interface, which severely limit long-term cycling stability. Here, we report a solvent-free surface-engineering strategy based on initiated chemical vapor deposition (iCVD) to construct a dual-functional interfacial architecture within the GDE. A hydrophilic poly-(glycidyl methacrylate) (poly-(GMA)) interlayer was conformally deposited at the electrolyte interface to enhance electrolyte uptake and ionic transport, while a hydrophobic poly-(2-(perfluorohexyl)-ethyl acrylate) (poly-(PFHEA)) layer was introduced on the air side to preserve gas permeability. The optimized poly-(GMA) coating exhibited high electrolyte uptake (291 ± 8%) and enhanced ionic conductivity (1.61 mS cm
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