ArticleAdvanced materials (Deerfield Beach, Fla.)2026
Topological Crosslinker Design Regulates Interfacial and Active Species Transport in Zinc-Iodine Batteries.
Article in Advanced materials (Deerfield Beach, Fla.), 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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Abstract
Aqueous zinc-ion batteries (ZIBs) are limited by interfacial instability and an intrinsic trade-off between mechanical strength and ionic conductivity in polymer gel electrolytes (PGEs), restricting their cycling durability and practical application. Here, we report a topology-regulated crosslinker strategy that redefines crosslinkers from passive structural components to active regulators of ion transport and interfacial chemistry. A tetra-armed poly(2-ethyl-2-oxazoline) (4-PEtOx) crosslinker is integrated into a zwitterionic network to construct a hydrogel electrolyte (4-PVEX). The unique molecular topology establishes a dense yet dynamic hydrogen-bonding framework, enabling continuous Zn
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