ArticleScience advances2026
Spiral-potato-like nanostructure COF enabling nearly unidirectional zinc deposition for Ah-level pouch cells.
Article in Science advances, 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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11 authors.
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Abstract
A major challenge in realizing ampere hour (Ah)-level aqueous zinc (Zn) ion pouch batteries (Ah-level AZIBs) is the requirements for high Zn utilization rate coupled with even Zn nucleation/growth. Here, we report a spiral-potato-like covalent organic framework (SP-COF) nanostructure to construct isotropic solid electrolyte interphase for Ah-level AZIBs. Compared with conventional COF nanostructures, the unique spiral-potato-like SP-COF combined with affinity sites and porosity enables isotropic interfacial regulation to achieve nearly unidirectional Zn deposition following the theoretical three-dimensional nucleation curve. As a result, symmetric cells based on SP-COF/Zn electrode display ultrastable plating/stripping over 2800 hours at 10 milliamperes per square centimeter. The successfully assembled Ah-level triple stacked layer pouch cell (SP-COF/Zn||I
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