Evidence map›Paper›PMID 42487498›Full record

ArticleAdvanced materials (Deerfield Beach, Fla.)2026

A Non-Equilibrium Flame Aerosol Process to Create High-Entropy MOFs.

Shuo Liu, Jiashun Liang, Mohd Ashhar Khan, Shaon Das, Jialu Li, Chao Zheng, Sanjit Ghose, Dominik Wierzbicki, Qike Jiang, Kaiwen Chen and 13 more

Abstract read
PubMed Full text at PMC Publisher
In one paragraph

Article in Advanced materials (Deerfield Beach, Fla.), 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.

0numbers the graph read from it
0cells of the map it votes in
0citing papers in PubMed
–field-weighted citation impact
1 · What the graph read from it

What it found

Each row is one number read from the abstract, on the scale the paper reported it, with its interval. Left of the dashed line favours the treatment, right favours the comparator. Under each row is the sentence it came from. New to these charts? A ten-minute tutorial.

The abstract states no effect estimate the extractor could read, or names no intervention and outcome on the map, so this paper lights no cell and moves no belief. It is still indexed, cited and linked below.

2 · The registry

The trial behind it

Trials whose registry record cites this paper, or whose number appears in the abstract. A trial that started after this paper was published is citing it as background, not reporting it.

Neither the registry nor the abstract names a trial number. If this is a trial report, that itself is worth knowing.

3 · Its place in the literature

Who cites it

0 citing papers in PubMed.

No citing paper in PubMed yet.

4 · The record

Corrections and comments

PubMed lists nothing against this paper. Absence here is not a guarantee, only a check that was made.

5 · Who and what money

Authors and funding

23 authors.

Shuo LiuDepartment of Chemical and Biological Engineering, University At Buffalo, The State University of New York, Buffalo, New York, USA.
Jiashun LiangDepartment of Chemical and Biological Engineering, University At Buffalo, The State University of New York, Buffalo, New York, USA.
Mohd Ashhar KhanDepartment of Chemical and Biological Engineering, University At Buffalo, The State University of New York, Buffalo, New York, USA.
Shaon DasDepartment of Materials Design and Innovation, University At Buffalo, The State University of New York, Buffalo, New York, USA.ORCID https://orcid.org/0000-0002-2160-6058
Jialu LiAdvanced Light Source, Lawrence Berkeley National Laboratory, Berkeley, California, USA.
Chao ZhengDepartment of Chemical and Biological Engineering, University At Buffalo, The State University of New York, Buffalo, New York, USA.
Sanjit GhoseNational Synchrotron Light Source ǁ, Brookhaven National Laboratory, Upton, New York, USA.
Dominik WierzbickiNational Synchrotron Light Source ǁ, Brookhaven National Laboratory, Upton, New York, USA.
Qike JiangInstrumentation and Service Center For Physical Sciences, Westlake University, Hangzhou, Zhejiang, China.
Kaiwen ChenDepartment of Chemical and Biological Engineering, University At Buffalo, The State University of New York, Buffalo, New York, USA.
Christina T ScalzoMagnetic Resonance Center, University At Buffalo, The State University of New York, Buffalo, New York, USA.
Zhengxi XuanDepartment of Chemical and Biological Engineering, University At Buffalo, The State University of New York, Buffalo, New York, USA.
Sai Varun KarepakulaDepartment of Chemical and Biological Engineering, University At Buffalo, The State University of New York, Buffalo, New York, USA.
Yaoli ZhaoDepartment of Chemical and Biological Engineering, University At Buffalo, The State University of New York, Buffalo, New York, USA.
Kun WangKazuo Inamori School of Engineering, Alfred University, New York, USA.
Jinghua GuoAdvanced Light Source, Lawrence Berkeley National Laboratory, Berkeley, California, USA.
Baishakhi MazumderDepartment of Materials Design and Innovation, University At Buffalo, The State University of New York, Buffalo, New York, USA.
Wei ChenDepartment of Materials Design and Innovation, University At Buffalo, The State University of New York, Buffalo, New York, USA.
Kaihang ShiDepartment of Chemical and Biological Engineering, University At Buffalo, The State University of New York, Buffalo, New York, USA.ORCID https://orcid.org/0000-0002-0297-1746
Gang WuDepartment of Chemical and Biological Engineering, University At Buffalo, The State University of New York, Buffalo, New York, USA.ORCID https://orcid.org/0000-0003-0885-6172
Jeffrey J UrbanThe Molecular Foundry, Lawrence Berkeley National Laboratory, Berkeley, California, USA.ORCID https://orcid.org/0000-0003-4909-2869
Mark T SwihartDepartment of Chemical and Biological Engineering, University At Buffalo, The State University of New York, Buffalo, New York, USA.
Chaochao DunThe Molecular Foundry, Lawrence Berkeley National Laboratory, Berkeley, California, USA.

Funding

Basic Energy SciencesDOE Buildings Technology Office DEEE-0008675National Energy Technology Laboratory DE-FE0032209National Science Foundation CBET-1804996Office of ScienceU.S. Department of Energy DE-AC02-05CH11231
6 · The paper itself

Abstract

High-entropy alloys and ceramics have demonstrated promising applications in the past decade. Ultrafast heating and cooling can kinetically trap immiscible elements into solid solutions, expanding the compositional space and optimizing the properties of high-entropy materials. However, the extreme temperatures required by these non-equilibrium methods are incompatible with metal-organic frameworks (MOFs). This work presents a flame aerosol strategy for synthesizing compositionally complex, entropically stabilized MOFs, enabling new combinations of properties previously inaccessible in this class of materials. Using the HKUST structure as a prototype, this methodology is extended to a wide array of both crystalline and amorphous MOFs, and then to a 10-element MOF that incorporates transition metals, rare-earth metals, alkaline-earth metals, p-block metals, and noble metals. This strategy can be further applied to inorganic coordination polymers. This study reveals that kinetics and entropy collectively drive structural short-range periodicity and configurational disorder in the framework, which in turn influence crystallinity, pore architecture, defect density, homogeneity, and electrochemical properties. This work expands the compositional design space for MOFs and offers new opportunities for their fundamental study and practical application.

Indexed as

flame spray pyrolysishigh‐entropy materialsMOFsnon‐equilibrium synthesis

Identifiers

PMID42487498
PMCPMC13532435

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Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.