ArticleNature communications2026
On the nature of chemical short-range order evolution.
Article in Nature communications, 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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Abstract
Chemical short-range order (CSRO), the non-random local arrangement of atoms in solid solutions, strongly affects the phase stability and performance of medium- and high-entropy alloys (M/HEAs). Despite its importance, the fundamental nature of CSRO formation remains contested: is it a formal thermodynamic transition? Here, investigating CoCrNi as a model system, we indicate that the main CSRO transformations observed in alloys might not be classical thermodynamic transitions, but instead a kinetic arrest phenomenon analogous to the glass transition. Combining atomistic simulations and in situ synchrotron dilatometry experiments enabled the study of CSRO evolution and its structural impact across multiple length scales. For example, CSRO-driven changes in bond lengths and bond distribution significantly impact the observed lattice parameter and volume, allowing Warren-Cowley parameter values to be determined over a full experimental temperature range. We demonstrate that the degree of CSRO and the apparent transition temperatures, defined here as the komplex reaction temperatures (T
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