ArticleSmall (Weinheim an der Bergstrasse, Germany)2026
Chemically Coupled Multifunctional Binder Networks Enable Stable and Safe Microscale Silicon Anodes.
Article in Small (Weinheim an der Bergstrasse, Germany), 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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Abstract
Silicon is a promising anode material for high-energy-density lithium-ion batteries due to its ultrahigh theoretical capacity; however, its practical applications are largely impeded by severe capacity fading induced by the substantial volume changes during the lithiation and delithiation process. Here, we report a flame-retardant polymeric binder with high stretchability that significantly enhances electrochemical performance and thermal safety of microscale silicon anodes. The multifunctional binder integrates rigid poly(acrylic acid) (PAA) as a mechanically robust framework and adenosine triphosphate (ATP) as active flame-retardant segments, with the two components chemically cross-linked via amidation. The resulting µSi/ATP-PAA electrode exhibits a high initial Coulombic efficiency of 89.33% and excellent long-term cycling stability, retaining a high specific capacity of 1427 mAh g
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