Evidence map›Paper›PMID 42454702›Full record

ArticleAdvanced materials (Deerfield Beach, Fla.)2026

Hydrogel-Woven COF Membranes With Orthogonal, Opposite Thermoresponsive Nanochannels: Overcoming the Permeance-Selectivity Trade-off.

Shuhui Ma, Hao-Nan Li, Chuang-Wei Gu, Cheng-Ye Zhu, Guang-Chang Xu, Mingxiu Lv, Chao Zhang, Zhi-Kang Xu

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In one paragraph

Article in Advanced materials (Deerfield Beach, Fla.), 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.

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0citing papers in PubMed
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1 · What the graph read from it

What it found

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The abstract states no effect estimate the extractor could read, or names no intervention and outcome on the map, so this paper lights no cell and moves no belief. It is still indexed, cited and linked below.

2 · The registry

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3 · Its place in the literature

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4 · The record

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5 · Who and what money

Authors and funding

8 authors.

Shuhui MaMOE Key Laboratory of Macromolecular Synthesis and Functionalization, Zhejiang Key Laboratory of Advanced Organic Materials and Technologies, Department of Polymer Science and Engineering, Zhejiang University, Hangzhou, China.
Hao-Nan LiMOE Key Laboratory of Macromolecular Synthesis and Functionalization, Zhejiang Key Laboratory of Advanced Organic Materials and Technologies, Department of Polymer Science and Engineering, Zhejiang University, Hangzhou, China.
Chuang-Wei GuMOE Key Laboratory of Macromolecular Synthesis and Functionalization, Zhejiang Key Laboratory of Advanced Organic Materials and Technologies, Department of Polymer Science and Engineering, Zhejiang University, Hangzhou, China.
Cheng-Ye ZhuMOE Key Laboratory of Macromolecular Synthesis and Functionalization, Zhejiang Key Laboratory of Advanced Organic Materials and Technologies, Department of Polymer Science and Engineering, Zhejiang University, Hangzhou, China.
Guang-Chang XuMOE Key Laboratory of Macromolecular Synthesis and Functionalization, Zhejiang Key Laboratory of Advanced Organic Materials and Technologies, Department of Polymer Science and Engineering, Zhejiang University, Hangzhou, China.
Mingxiu LvMOE Key Laboratory of Macromolecular Synthesis and Functionalization, Zhejiang Key Laboratory of Advanced Organic Materials and Technologies, Department of Polymer Science and Engineering, Zhejiang University, Hangzhou, China.
Chao ZhangMOE Key Laboratory of Macromolecular Synthesis and Functionalization, Zhejiang Key Laboratory of Advanced Organic Materials and Technologies, Department of Polymer Science and Engineering, Zhejiang University, Hangzhou, China.
Zhi-Kang XuMOE Key Laboratory of Macromolecular Synthesis and Functionalization, Zhejiang Key Laboratory of Advanced Organic Materials and Technologies, Department of Polymer Science and Engineering, Zhejiang University, Hangzhou, China.

Funding

Fundamental Research Funds for the Central Universities 226-2024-00027Fundamental Research Funds for the Central Universities 226-2025-00011National Natural Science Foundation of China 22375174Natural Science Foundation of Zhejiang Province LZ24E030001
6 · The paper itself

Abstract

Smart membranes, characterized by unique stimuli-responsive channels to dynamically alter their chemistry and structure for orchestrating mass transport, are highly promising to gain extraordinary sieving performance over conventional membranes. However, smart membranes are locked by formidable trade-off between permeance and selectivity during stimuli-responsive process, owing to their synchronous, homogeneous stimuli-responsive changes in channels. Here, we discover a new kind of smart membranes, hydrogel-woven covalent organic framework (HW-COF) membranes with orthogonal, opposite thermoresponsive nanochannels, overcoming the permeance-selectivity trade-off for achieving extraordinary aqueous separation. The key of HW-COF membranes lies in the photothermal-driven in-situ confined weaving of poly(N-isopropylacrylamide) hydrogel networks within orthogonal in-plane pores and interlayer channels of two-dimensional COF membranes for yielding mechanical interlocking architecture. Distinct from the non-interlocked counterpart, HW-COF membranes showcase a positive response in in-plane pores yet a negative response in interlayer channels. This unique thermoresponsive behavior can be tailored by the synergy of in-plane pores and interlayer channels, allowing HW-COF membranes to obtain markedly positive response in both permeance and selectivity, almost not achievable with reported smart membranes. As a concept of demonstration, HW-COF membranes can be applied for sieving water isotopologue with ultrahigh selectivity (90.9%) and permeance (16.6 L m

Indexed as

covalent organic frameworkshydrogelmembrane separationphotothermal in situ weaving

Identifiers

PMID42454702
PMCPMC13471893

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