ArticleChemical science2026
Terahertz dynamics at the actinide frontier: linking low-frequency vibrations, electronic structure, and bonding in molecular uranium complexes.
Article in Chemical science, 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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Abstract
Understanding the nature of uranium-ligand bonding in molecular complexes is a central challenge in modern actinide chemistry. Here, we introduce low-frequency vibrational spectroscopy as a powerful new probe of bonding in uranium-containing molecular crystals by combining terahertz and low-frequency Raman spectroscopy with periodic solid-state density functional theory simulations. Using U(vi)(O
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