ArticleAdvanced materials (Deerfield Beach, Fla.)2026
Inorganic Ionic Polymerization-Anchored Polymer Networks for Ultrastrong and Ultratough Eutectogels.
Article in Advanced materials (Deerfield Beach, Fla.), 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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Abstract
Eutectogels hold considerable promise for applications in flexible electronics, soft robotics, and protective systems owing to their combination of the environmental stability of deep eutectic solvents and the mechanical robustness of polymer networks. However, predominantly weak intermolecular interactions among polymer chains within eutectogels restrict their mechanical performance, making it challenging to simultaneously achieve high strength and high toughness. Herein, we propose an inorganic ionic polymerization-anchored polymer network (IIP-APN) strategy to construct ultrastrong and ultratough eutectogels. Specifically, calcium phosphate oligomers (CPO) are incorporated into the polyvinyl alcohol (PVA) chain network to serve as nanoanchors. Through inorganic ionic polymerization, hydroxyapatite nanorivets are generated to anchor PVA chains, forming a hierarchically integrated organic-inorganic composite network. This unique riveting network structure imparts record-breaking ultrahigh toughness (696.4 ± 119.1 MJ m
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