ArticleAngewandte Chemie (International ed. in English)2026
Intramolecularly Synergic Catalysis Enables Efficient Closed-Loop Recycling of Polyesters and Polycarbonates.
Article in Angewandte Chemie (International ed. in English), 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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Abstract
Efficient and selective chemical recycling of commercial plastics back to monomers is a pivotal strategy for achieving a circular plastics economy. However, rare catalysts can deliver versatility in both polymerization and depolymerization processes. Herein, we report an efficient and tolerant dinuclear zinc catalyst for the bulk depolymerization of various polyesters and polycarbonates to the corresponding cyclic monomers with >99% selectivity, and for repolymerization to virgin materials, through an intramolecular bimetallic synergistic dual-activation mechanism. A record-breaking activity of up to 43 kg of polymer/g of catalyst per hour was observed in the catalytic bulk poly(
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