ArticleAdvanced materials (Deerfield Beach, Fla.)2026
Chain-Mobility-Enabled 1D Lanthanide Coordination Polymer Glassy Scintillators for Underwater X-Ray Videography.
Article in Advanced materials (Deerfield Beach, Fla.), 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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Abstract
Lanthanide(III) coordination scintillators feature efficient triplet harvesting and narrow-band emission, making them promising for X-ray imaging applications. However, their rigid coordination environments hinder melt-processing into large-area, transparent glassy scintillator screens. Herein, a "rigid-node flexible-linker" molecular design strategy that facilitates chain-mobility-enabled glass-forming in lanthanide coordination scintillators by constructing one-dimensional (1D) coordination chains is proposed. By integrating dibenzoylmethane antenna with flexible dual-phosphine-oxide linkers (OP-Cn, n = 2, 4, 6, 8), a series of 1D Eu-OP-Cn coordination polymers is constructed, enabling the simultaneous realization of efficient ligand-sensitized radioluminescence and the chain-mobility required for vitrification, thereby allowing transformation from crystalline powders into glassy states. Benefiting from rigid local coordination environments that suppress nonradiative decay, crystalline Eu-OP-C2 exhibits a near-unity photoluminescence quantum yield (97.5%) and an ultrahigh relative light yield of 70379 photons MeV
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