ArticleMacromolecular rapid communications2026
From Molecular Structure to Macroscopic Performance: Insights into Polycarbosilane Curing.
Article in Macromolecular rapid communications, 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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7 authors.
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Abstract
Curing protocols critically influence the structure and properties of crosslinked polymer networks, yet their impact on nanoscale structural features remains poorly understood. Here, polycarbosilane (PCS) networks are used as a model system to investigate curing-induced structural evolution across multiple techniques. PCS networks were prepared via Pt-catalyzed hydrosilylation reaction at progressively higher curing temperatures, and their macroscopic properties were correlated with molecular-level changes using a combined experimental-computational approach. Mechanical testing revealed a transition from flexible to brittle behavior with increasing curing temperature, while dynamic mechanical thermal analysis (DMTA) and swelling experiments showed a continuous increase in glass transition temperature (T
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