ArticleSmall (Weinheim an der Bergstrasse, Germany)2026
Finding the Perfect Match: Investigation of 1,2-Diketone-Based Materials for Use as Cathode Active Material in Rechargeable Magnesium Batteries.
Article in Small (Weinheim an der Bergstrasse, Germany), 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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Abstract
Motivated by the high capacity and energy enabled by the two-electron donation of earth-abundant magnesium, we developed a novel, generally applicable screening method to evaluate 1,2-diketone-based redox units as n-type cathode active materials (CAMs) for rechargeable magnesium batteries (RMBs). Preliminary DFT calculations (redox potentials, charge density mapping) and cyclic voltammetry in supporting and magnesium electrolyte solutions were used to screen exemplary diketone classes, eliminating unsuitable candidates and identifying phenanthrenequinone (PNQ) as the most promising redox unit for incorporation into a vinylic polymer. Non-conjugated PNQ-based vinylic polymers were successfully synthesized, characterized, and tested as CAMs at the coin-cell level. Non-optimized Mg-PNQ cells delivered a starting capacity of up to 77 mAh g
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