ArticleSmall (Weinheim an der Bergstrasse, Germany)2026
3DOM POM@MOF-Enhanced Polymer Electrolytes Enabling Dendrite-Suppressed, High-Performance All-Solid-State Lithium-Metal Battery.
Article in Small (Weinheim an der Bergstrasse, Germany), 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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Abstract
All-solid-state lithium batteries (ASSLBs) provide high energy density and improved safety but remain limited by lithium dendrite formation and low ionic conductivity at room temperature. This work reports an effective strategy to address these issues by incorporating hierarchically ordered macro/microporous polyoxometalate-based metal-organic frameworks (3DOM POM@MOFs), specifically 3DOM NENU-3a, into a polyethylene oxide (PEO) matrix to form a composite solid electrolyte (CSE). The three-dimensionally ordered macroporous structure, prepared via a hard-template method, preserves the advantages of microporous POM@MOFs while introducing interconnected macropores that enhance ion transport. With only 1 wt.% 3DOM NENU-3a added to a PEO/lithium bis(trifluoromethanesulfonyl)imide (LiTFSI) system, the resulting CSE exhibits high ionic conductivity (1.32 × 10
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