ArticleAngewandte Chemie (International ed. in English)2026
Crystalline Small Molecule-Polymer Superlattice for Spatially Isolated Tetrathiafulvalene Spin Qubit Arrays.
Article in Angewandte Chemie (International ed. in English), 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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Abstract
Molecular electron spins are compelling qubit candidates; however, mitigating their rapid relaxation and decoherence driven by structural disorder and phonon coupling remains a central challenge. Constructing molecular qubit frameworks (MQFs) represents a promising strategy to preserve quantum coherence by embedding spin centers in a rigid and ordered microenvironment. Here, we report a host-guest superlattice MQF by cocrystallizing tetrathiafulvalene (TTF) with a one-dimensional B←N coordination polymer (CityU-65). Encaging TTF radical spins within this highly ordered lattice establishes a rigid and magnetically dilute environment, effectively suppressing spin-lattice relaxation and partially mitigating spin decoherence. Consequently, CityU-65 preserves coherent spin addressability even under ambient conditions. At room temperature, the superlattice exhibits a prolonged spin-lattice relaxation time (T
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