ArticleChemical science2026
Kinetically programmed pathway-dependent autonomous reversibility in biomimetic self-assembly of nanoparticles.
Article in Chemical science, 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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3 authors.
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Abstract
Autonomous reversibility is fundamental to many natural systems, enabling the formation of dynamic and adaptive assemblies without continuous external intervention. Replicating autonomous behavior in artificial systems remains challenging, as it demands a kinetic imbalance in the self-assembly process driven by chemically triggered dynamic interactions. Here, we demonstrate pathway-dependent autonomous reversibility in a bio-nano hybrid system composed of adenosine triphosphate (ATP) and gold nanoparticles (AuNPs), with hexokinase (HK) as an enzymatic disassembling trigger. The electrostatic interaction between oppositely charged AuNPs and ATP drives co-assembly, while HK-mediated dephosphorylation of ATP to ADP weakens these interactions, inducing rapid disassembly. Autonomous reversibility is achieved
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