ArticleThe journal of physical chemistry letters2026
Lithium-Ion Partial Molar Entropies in Liquid, Composite, and Solid-State Electrolytes.
Article in The journal of physical chemistry letters, 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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Abstract
Electrolyte composition, concentration, and structure can affect reaction kinetics, ion transport, and heat generation during operation. In liquid electrolyte systems, the properties of ion-solvent and ion-ion interactions strongly affect thermodynamics and electrochemistry. The change in total entropy of the electrolyte when one mole of an ion is added to an electrolyte at a constant temperature and pressure is known as the partial molar entropy of ion solvation and describes broadly how the solvation environment changes with the addition or removal of an ion. Herein, we measure the partial molar entropies of lithium-ion solvation in solid-state systems using potentiometric temperature coefficient measurements. For solid-state systems, we measure positive partial molar entropies of lithium-ion solvation of 43.3 J mol
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