ArticleAdvanced materials (Deerfield Beach, Fla.)2026
Light-Induced Proton Transfer Tautomeric Frustrated Lewis Pairs on Carbon Nitride.
Article in Advanced materials (Deerfield Beach, Fla.), 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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Abstract
The static nature of active sites in heterogeneous frustrated Lewis pairs (FLPs) often limits their adaptability and efficiency in dynamic catalytic environments. Challenges such as the inevitable quenching of sites at high loadings and vulnerability to poisoning restrict their practical application. Inspired by the inherent dynamicity of soft materials, we report a paradigm shift from static design to light-regulated dynamic catalysis by constructing Tautomeric Frustrated Lewis Pairs (TFLPs) on carbon nitride frameworks. Through supramolecular self-assembly, we engineered carbon nitride isomers capable of undergoing photoinduced keto-enol and phosphinylidene tautomerization. This process in situ generates transient, yet stabilized, electron-deficient (Lewis acid) and electron-rich (Lewis base) sites with appropriate spatial frustration. This dynamic system was employed in the photocatalytic oxidation of H
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