In Situ Synchronized SERS-SEIRAS Unveils Cation-Regulated Interfacial Water and Intermediates in the Oxygen Reduction Reaction.

Xiao-Xuan Huang, Yao-Hui Wang, Jianmin Su, Ling-Yun Hu, Hong-Jia Wang, Jia-Sheng Lin, Xia-Guang Zhang, Jian-Feng Li

Abstract read

In one paragraph

Article in Angewandte Chemie (International ed. in English), 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.

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1 · What the graph read from it

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5 · Who and what money

Authors and funding

8 authors.

Xiao-Xuan HuangCollege of Materials, State Key Laboratory of Physical Chemistry of Solid Surfaces, iChEM, College of Chemistry and Chemical Engineering, College of Energy, and College of Physical Science and Technology, Xiamen University, Xiamen, China.

Yao-Hui WangCollege of Materials, State Key Laboratory of Physical Chemistry of Solid Surfaces, iChEM, College of Chemistry and Chemical Engineering, College of Energy, and College of Physical Science and Technology, Xiamen University, Xiamen, China.

Jianmin SuCollege of Materials, State Key Laboratory of Physical Chemistry of Solid Surfaces, iChEM, College of Chemistry and Chemical Engineering, College of Energy, and College of Physical Science and Technology, Xiamen University, Xiamen, China.

Ling-Yun HuCollege of Materials, State Key Laboratory of Physical Chemistry of Solid Surfaces, iChEM, College of Chemistry and Chemical Engineering, College of Energy, and College of Physical Science and Technology, Xiamen University, Xiamen, China.

Hong-Jia WangCollege of Materials, State Key Laboratory of Physical Chemistry of Solid Surfaces, iChEM, College of Chemistry and Chemical Engineering, College of Energy, and College of Physical Science and Technology, Xiamen University, Xiamen, China.

Jia-Sheng LinCollege of Chemical Engineering and Materials Science, Quanzhou Normal University, Quanzhou, China.

Xia-Guang ZhangKey Laboratory of Green Chemical Media and Reactions, Ministry of Education, Collaborative Innovation Center of Henan, Province for Green Manufacturing of Fine Chemicals, School of Chemistry and Chemical Engineering, Henan Normal University, Xinxiang, China.ORCID https://orcid.org/0000-0002-9223-0852

Jian-Feng LiCollege of Materials, State Key Laboratory of Physical Chemistry of Solid Surfaces, iChEM, College of Chemistry and Chemical Engineering, College of Energy, and College of Physical Science and Technology, Xiamen University, Xiamen, China.ORCID https://orcid.org/0000-0003-1598-6856

Funding

Fundamental Research Funds for the Central Universities 20720240054Industry-University-Research Joint Innovation Project of Fujian Province 2025H6023Liaoning Binhai Laboratory 2024-05National Natural Science Foundation of China 22322206National Natural Science Foundation of China 22361132532National Natural Science Foundation of China 22472141National Natural Science Foundation of China 22474116National Natural Science Foundation of China 22525042National Natural Science Foundation of China T2293692New Cornerstone Science Foundation through the XPLORER PRIZEScientific and Technological Project of Yunnan Precious Metals Laboratory YPML-20240502063State Key Laboratory of Fine Chemicals, Dalian University of Technology KF2401

6 · The paper itself

Abstract

Interfacial water plays a crucial yet poorly understood role in the alkaline oxygen reduction reaction (ORR) by modulating the adsorption of oxygen intermediates and mediating proton-coupled electron transfer (PCET). However, the lack of techniques to dynamically correlate interfacial water with adsorbed intermediates makes it difficult to elucidate the mechanism governing the evolution of intermediate species. Here, we report a synchronized, site-consistent SERS-SEIRAS platform that tracks interfacial water and surface-adsorbed species (OOH

Indexed as

cation effectinterfacial waterORR performanceoxygen intermediatesSERS‐SEIRAS coupling

Identifiers

PMID42287653

DOI10.1002/anie.8900381

PMCPMC13480511

What OpenQuestion holds

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Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.