ArticleMaterials (Basel, Switzerland)2026
Molecular Design of Underwater Adhesive Copolymers: Synergy Between Long-Chain Alkyl Crystallization-Melting Switching and Carboxyl Group Interfacial Interactions.
Article in Materials (Basel, Switzerland), 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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Abstract
Achieving strong adhesion in underwater or humid environments remains challenging because the interfacial hydration layer prevents direct contact between the adhesive and the substrate. Conventional adhesives typically fail under these conditions, so new strategies are needed to actively displace the water layer and create stable interfacial interactions. In this study, we prepared a series of copolymers with different monomer ratios via photocuring, using methacrylic acid (MAA) and stearyl methacrylate (SMA) as monomers. We focused on their thermal transition behavior and adhesion performance under both dry and underwater conditions. The results show that at an SMA molar fraction of 85%, the copolymer exhibits crystalline melting between 30 and 40 °C, where the storage modulus drops from approximately 10
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