ArticleCommunications chemistry2026
Discovery of a low-density filled-ice phase in nitrogen hydrate at high pressure.
Article in Communications chemistry, 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 1 paper.
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1 citing paper in PubMed.
- Free Energy Differences and Coexistence of Clathrate Structures II and H via Lattice-Switch Monte Carlo.Journal of chemical theory and computation · 2026Article
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10 authors.
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Abstract
Nitrogen, Earth's most abundant atmospheric component, in the presence of water, is known to form clathrate hydrates, that are relevant to model the evolution of water-rich planets and satellites. Here, we map the high-pressure phase diagram of nitrogen hydrate up to 16 GPa at room temperature by combining neutron diffraction, Raman spectroscopy, and crystal structure prediction. We reveal a rich sequence of structural transformations, from sI/sII clathrates to hexagonal (sH) and tetragonal (sT) phases, culminating in a previously unknown orthorhombic filled-ice structure above 1.8 GPa. This new phase cannot be indexed to any known ice frameworks and exhibits a density approximately 30% lower than that of stable ice VII, pointing to distinctive water-nitrogen interactions. Our results refine the understanding of nitrogen hydrate behavior under extreme conditions and demonstrate the propensity of N
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