ArticleAngewandte Chemie (International ed. in English)2026
Ammonia-Resistant Carbon-Encapsulated Cobalt Catalyst for Electrocatalytic Nitrate Reduction to Volatile Ammonia.
Article in Angewandte Chemie (International ed. in English), 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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Abstract
Electrocatalytic nitrate reduction to ammonia presents a promising route for sustainable nitrogen utilization; however, current efforts remain largely confined to optimizing synthesis efficiency, with insufficient attention paid to the concurrent challenge of ammonia separation-a key bottleneck for scalable deployment. Here, we report carbon-shell-encapsulated cobalt nanoparticles (Co@C), which uniquely enable integrated ammonia synthesis and in situ gas-phase purification under strongly alkaline conditions. In both sequencing batch and continuous-flow electrolyzers, Co@C delivers a robust nitrate-to-ammonia Faradaic efficiency of 92.4%, maintaining performance even in the presence of exogenous ammonia. Critically, the high-pH environment shifts the NH
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