High-Energy-Facet-Oriented Mesoporous Single-Crystal Metal Oxides for Selective Oxidation Catalysis.

Yangbo Dong, Tao Wang, Wei Li, Yan Song, Shuzhen Dou, Yan Yang, Ling Zhang, Zhen-An Qiao

Abstract read

In one paragraph

Article in Advanced materials (Deerfield Beach, Fla.), 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.

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5 · Who and what money

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8 authors.

Yangbo DongState Key Laboratory of Inorganic Synthesis and Preparative Chemistry, College of Chemistry, Jilin University, Changchun, Jilin, P. R. China.

Tao WangState Key Laboratory of Inorganic Synthesis and Preparative Chemistry, College of Chemistry, Jilin University, Changchun, Jilin, P. R. China.ORCID https://orcid.org/0000-0001-5004-160X

Wei LiState Key Laboratory of Inorganic Synthesis and Preparative Chemistry, College of Chemistry, Jilin University, Changchun, Jilin, P. R. China.

Yan SongState Key Laboratory of Inorganic Synthesis and Preparative Chemistry, College of Chemistry, Jilin University, Changchun, Jilin, P. R. China.

Shuzhen DouJiangxi Academy of Sciences, Nanchang, Jiangxi, P. R. China.

Yan YangState Key Laboratory of Inorganic Synthesis and Preparative Chemistry, College of Chemistry, Jilin University, Changchun, Jilin, P. R. China.

Ling ZhangState Key Laboratory of Supramolecular Structure and Materials, College of Chemistry, Jilin University, Changchun, Jilin, P. R. China.ORCID https://orcid.org/0000-0001-5511-1136

Zhen-An QiaoState Key Laboratory of Inorganic Synthesis and Preparative Chemistry, College of Chemistry, Jilin University, Changchun, Jilin, P. R. China.ORCID https://orcid.org/0000-0001-6064-9360

Funding

"111" Project of the Ministry of Education of China B17020Jilin Province Science and Technology Development Plan 20260602006RCNational Key R&D Program of China 2023YFA1506301National Natural Science Foundation of China 22175071National Natural Science Foundation of China 22402109National Natural Science Foundation of China 22425104Program for Young Scholar Talents of Wenying in Shanxi UniversityScience and Technology Innovation Project of Shanxi Province Higher Education Institutions 2024L013

6 · The paper itself

Abstract

Mesoporous single-crystal metal oxides are highly attractive for heterogeneous catalysis because they combine high surface accessibility with long-range lattice coherence; however, their synthesis remains fundamentally challenging due to the thermodynamic incompatibility between crystallization and pore formation. Here we report a template-free, energy-driven facet-oriented crystallization strategy that enables the formation of mesoporous single-crystal metal oxides with tunable pore architectures and exposed high-energy facets. Polyvinylpyrrolidone functions simultaneously as a pore maintainer and surface-energy regulator, preserving mesoporosity while selectively stabilizing high-energy facets to direct single-crystal growth. The method is applicable to multiple oxides, including Co

Indexed as

mesoporousmetal oxidesselective oxidationsingle‐crystal

Identifiers

PMID42261069

DOI10.1002/adma.73641

PMCPMC13361156

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Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.